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Single atom solutions for carbon dioxide capture

  • Chen Zhang
  • , Chenyang Zhou
  • , Yuan Li
  • , Yunsong Yu
  • , Jingfeng Zhang
  • , Zaoxiao Zhang
  • , Geoff Wang
  • Xi'an Jiaotong University
  • University of Queensland

科研成果: 期刊稿件文章同行评审

23 引用 (Scopus)

摘要

New solvents are considered to be one of the effective methods to facilitate the reaction rate and lower the reaction energy barrier. However, the common method to develop a new solvent has come to a dead end. Thus, a single atom in solvent to produce a single atom solution is designed to create the breakthrough. Eight kinds of single atom solutions are prepared as new absorbents. Experiments prove the single atom in the solutions and their charge-producing effects. A density functional theory model is developed to analyze the microscale characteristics. Meanwhile, it has been applied in carbon dioxide capture. The CO2 desorption rate is intensified in the single atom solution system due to the controlled reaction energy barrier. The results show that single atom solutions produce a maximum voltage of 2.12 V and, thus, contribute to near zero energy consumption by effectively harvesting the substantial waste heat below 373 K.

源语言英语
文章编号084309
期刊Journal of Chemical Physics
158
8
DOI
出版状态已出版 - 28 2月 2023

联合国可持续发展目标

此成果有助于实现下列可持续发展目标:

  1. 可持续发展目标 7 - 经济适用的清洁能源
    可持续发展目标 7 经济适用的清洁能源

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