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Physical Limit of Nonlinear Brownian Oscillators in Quantum Trap

  • Fangyuan Chen
  • , Zepu Kou
  • , Zonghuiyi Jiang
  • , Wanlin Guo
  • , Xiaofei Liu
  • Nanjing University of Aeronautics and Astronautics

科研成果: 期刊稿件文章同行评审

4 引用 (Scopus)

摘要

Quantum trap, a quantum and thermal fluctuations-induced nonmonotonous potential, offers a chance to build up microscopic mechanical systems completely dominated by fluctuations. Here, we explore the physical limit of the effective damping ratio of the nonlinear Brownian oscillator in a quantum trap, set by the finite separation for avoiding molecular-scale effects on the trap potential and the surface confinement effect-induced diverging damping and random forces. The quasiharmonic approximations and Langevin dynamics simulations show that the lowest effective damping ratios of the suspended Au plate and Au sphere upon a Teflon coating of 10 nm can be ∼210 and ∼145, respectively, at room temperature. Perforation is proposed as an effective route to reduce the damping ratio (down to 6.4) by attenuating the surface confinement effect. An unexpected result due to the temperature dependences of dielectric function and viscosity of ethanol is a further reduced damping ratio at 400 K (1.3). The nonlinear Brownian oscillator in the quantum trap shows promise of probing near-boundary hydrodynamics at nanoscale.

源语言英语
页(从-至)1719-1725
页数7
期刊Journal of Physical Chemistry Letters
15
6
DOI
出版状态已出版 - 15 2月 2024
已对外发布

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