Lagrangian Identification of Coherent Structures and Mass Transport in a Buoyant Jet Diffusion Flame

Using Lagrangian coherent structures (LCSs), the mass transport process of large-scale coherent structures in a buoyant jet diffusion flame is studied numerically to gain a key understanding of combustion instability. First, the reacting flow fields of the jet diffusion flame are numerically simulated for two cases, a stable case without considering the buoyancy effect and an unstable case that includes the buoyancy effect corresponding to combustion instability. In particular, large-scale Kelvin-Helmholtz instability (KHI) vortex structures outside the flame surface are captured in the unstable case. Then, the ridges in finite-time Lyapunov exponent (FTLE) fields that sketch the distinct regions in the reacting flow field are extracted as LCSs. The mass transport process is studied by comparing the distribution of LCSs with reaction fields. The flame surface is found to coincide with the attracting LCSs, which separate the fuel and air on opposite sides of the flame surface. In contrast, the reaction products, including species and reaction heat, are confined in the boundaries consisting of repelling LCSs on the inner and outer sides of the flame surface. Finally, the evolution of LCSs is tracked to analyze the generation of KHI vortices and species transport in the jet diffusion flame. With the aid of LCSs, it is found that there exist some saddle-type flow features separating the distinct flow structures into several regions, and the jet fuel and airflow enter into the separated regions from different open boundaries. Importantly, the attracting LCSs in the separated regions then bulge outwards, forming KHI vortices as the attracting LCSs further stretch and fold. Furthermore, the vortices continue moving upwards while species flow from repelling LCSs to attracting LCSs, leading to mixing. These results show that attracting and repelling LCSs can act as the flame surface and the mass and energy transport boundary of the reaction products, respectively. In summary, the work presented can provide a new method in combustion controlling to estimate the location of the flame surface and the transport boundaries of species from the velocity field, by using LCSs.