TY - JOUR
T1 - Electrospark-Induced Bubble Rupture for Micronano Bubble Formation in Water
AU - Zhu, Mengying
AU - Zhang, Mingyan
AU - Wang, Xiaoran
AU - Liu, Chenyu
AU - Zhou, Rusen
AU - Sun, Jing
AU - Zhou, Renwu
AU - Liu, Dingxin
N1 - Publisher Copyright:
© 2025 American Chemical Society
PY - 2025
Y1 - 2025
N2 - The generation of micronano bubbles (MNBs) typically relies on cavitation processes. However, discharge inside an underwater bubble causes bubble deformation, providing a new avenue for MNB formation. This study introduces a novel mechanism for micronano bubbles (MNB) generation through self-sustained discharge processes with underwater bubbles. High-speed imaging reveals the dynamic interplay between spark discharge formation and bubble structural evolution. A local thermal equilibrium (LTE) plasma model provides insights into the thermal and electrical dynamics during bubble rupture. The model demonstrates that, local temperature increases, up to 1750 K of a plasma gas temperature, resulting from discharge streamer activity within bubble cavities. Velocity streamlines near the bubble neck following its expansion at elevated temperatures indicate the initial position of the bubble breakup. The MNBs significantly enhance the dissolution and generation of reactive species, including O3and H2O2in the solution, highlighting their potential to enhance interfacial reactions and water disinfection applications.
AB - The generation of micronano bubbles (MNBs) typically relies on cavitation processes. However, discharge inside an underwater bubble causes bubble deformation, providing a new avenue for MNB formation. This study introduces a novel mechanism for micronano bubbles (MNB) generation through self-sustained discharge processes with underwater bubbles. High-speed imaging reveals the dynamic interplay between spark discharge formation and bubble structural evolution. A local thermal equilibrium (LTE) plasma model provides insights into the thermal and electrical dynamics during bubble rupture. The model demonstrates that, local temperature increases, up to 1750 K of a plasma gas temperature, resulting from discharge streamer activity within bubble cavities. Velocity streamlines near the bubble neck following its expansion at elevated temperatures indicate the initial position of the bubble breakup. The MNBs significantly enhance the dissolution and generation of reactive species, including O3and H2O2in the solution, highlighting their potential to enhance interfacial reactions and water disinfection applications.
UR - https://www.scopus.com/pages/publications/105018904719
U2 - 10.1021/acs.jpclett.5c02525
DO - 10.1021/acs.jpclett.5c02525
M3 - 文章
C2 - 41102993
AN - SCOPUS:105018904719
SN - 1948-7185
VL - 16
SP - 11101
EP - 11108
JO - Journal of Physical Chemistry Letters
JF - Journal of Physical Chemistry Letters
ER -