Constructing electron transport channel of SnO2/BaSO4 on g-C3N4 for enhanced visible-light-driven photocatalytic H2 production

Gongyue Dong; Xiaojuan Guo; Cheng Cheng; Feng Chen; Jinfeng Zhang; Yanping Du; Wei Meng; Maochang Liu; Jinwen Shi

doi:10.1016/j.mtcata.2025.100098

Constructing electron transport channel of SnO₂/BaSO₄ on g-C₃N₄ for enhanced visible-light-driven photocatalytic H₂ production

Gongyue Dong
, Xiaojuan Guo
, Cheng Cheng
, Feng Chen
, Jinfeng Zhang
, Yanping Du
, Wei Meng
, Maochang Liu
, Jinwen Shi

能源与动力工程学院

Xi'an Jiaotong University
Dongguan University of Technology
Gansu Company
Lancaster University
Hunan City University

科研成果: 期刊稿件 › 文章 › 同行评审

5 引用（Scopus）

摘要

Graphitic carbon nitride (g-C₃N₄) is confronted with the issue of poor utilization of photogenerated charge carriers, thereby leading to limited performance of photocatalytic hydrogen (H₂) production, which restricts its potential application. Herein, the electron transport material SnO₂/BaSO₄ was synthesized to integrate with g-C₃N₄ for addressing the above problem. Various characterizations were conducted to investigate the g-C₃N₄-SnO₂/BaSO₄ photocatalyst, and it demonstrated that photogenerated electrons from g-C₃N₄ expeditiously migrate to SnO₂/BaSO₄ nanoparticles, which markedly hindered photogenerated carriers’ recombination. Subsequently, the g-C₃N₄-SnO₂/BaSO₄ photocatalyst demonstrated promoted photocatalytic H₂ production at a rate of 14.2 μmol h⁻¹ under visible-light illumination, which was 2.5 times higher than that of pristine g-C₃N₄.

源语言	英语
文章编号	100098
期刊	Materials Today Catalysis
卷	9
DOI	https://doi.org/10.1016/j.mtcata.2025.100098
出版状态	已出版 - 6月 2025

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10.1016/j.mtcata.2025.100098

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title = "Constructing electron transport channel of SnO2/BaSO4 on g-C3N4 for enhanced visible-light-driven photocatalytic H2 production",

abstract = "Graphitic carbon nitride (g-C3N4) is confronted with the issue of poor utilization of photogenerated charge carriers, thereby leading to limited performance of photocatalytic hydrogen (H2) production, which restricts its potential application. Herein, the electron transport material SnO2/BaSO4 was synthesized to integrate with g-C3N4 for addressing the above problem. Various characterizations were conducted to investigate the g-C3N4-SnO2/BaSO4 photocatalyst, and it demonstrated that photogenerated electrons from g-C3N4 expeditiously migrate to SnO2/BaSO4 nanoparticles, which markedly hindered photogenerated carriers{\textquoteright} recombination. Subsequently, the g-C3N4-SnO2/BaSO4 photocatalyst demonstrated promoted photocatalytic H2 production at a rate of 14.2 μmol h−1 under visible-light illumination, which was 2.5 times higher than that of pristine g-C3N4.",

keywords = "Barium sulfate, Electron transport material, Graphitic carbon nitride, Photocatalysis, Tin dioxide",

author = "Gongyue Dong and Xiaojuan Guo and Cheng Cheng and Feng Chen and Jinfeng Zhang and Yanping Du and Wei Meng and Maochang Liu and Jinwen Shi",

note = "Publisher Copyright: {\textcopyright} 2025 The Authors",

year = "2025",

month = jun,

doi = "10.1016/j.mtcata.2025.100098",

language = "英语",

volume = "9",

journal = "Materials Today Catalysis",

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TY - JOUR

T1 - Constructing electron transport channel of SnO2/BaSO4 on g-C3N4 for enhanced visible-light-driven photocatalytic H2 production

AU - Dong, Gongyue

AU - Guo, Xiaojuan

AU - Cheng, Cheng

AU - Chen, Feng

AU - Zhang, Jinfeng

AU - Du, Yanping

AU - Meng, Wei

AU - Liu, Maochang

AU - Shi, Jinwen

PY - 2025/6

Y1 - 2025/6

N2 - Graphitic carbon nitride (g-C3N4) is confronted with the issue of poor utilization of photogenerated charge carriers, thereby leading to limited performance of photocatalytic hydrogen (H2) production, which restricts its potential application. Herein, the electron transport material SnO2/BaSO4 was synthesized to integrate with g-C3N4 for addressing the above problem. Various characterizations were conducted to investigate the g-C3N4-SnO2/BaSO4 photocatalyst, and it demonstrated that photogenerated electrons from g-C3N4 expeditiously migrate to SnO2/BaSO4 nanoparticles, which markedly hindered photogenerated carriers’ recombination. Subsequently, the g-C3N4-SnO2/BaSO4 photocatalyst demonstrated promoted photocatalytic H2 production at a rate of 14.2 μmol h−1 under visible-light illumination, which was 2.5 times higher than that of pristine g-C3N4.

AB - Graphitic carbon nitride (g-C3N4) is confronted with the issue of poor utilization of photogenerated charge carriers, thereby leading to limited performance of photocatalytic hydrogen (H2) production, which restricts its potential application. Herein, the electron transport material SnO2/BaSO4 was synthesized to integrate with g-C3N4 for addressing the above problem. Various characterizations were conducted to investigate the g-C3N4-SnO2/BaSO4 photocatalyst, and it demonstrated that photogenerated electrons from g-C3N4 expeditiously migrate to SnO2/BaSO4 nanoparticles, which markedly hindered photogenerated carriers’ recombination. Subsequently, the g-C3N4-SnO2/BaSO4 photocatalyst demonstrated promoted photocatalytic H2 production at a rate of 14.2 μmol h−1 under visible-light illumination, which was 2.5 times higher than that of pristine g-C3N4.

KW - Barium sulfate

KW - Electron transport material

KW - Graphitic carbon nitride

KW - Photocatalysis

KW - Tin dioxide

UR - https://www.scopus.com/pages/publications/105001048765

U2 - 10.1016/j.mtcata.2025.100098

DO - 10.1016/j.mtcata.2025.100098

M3 - 文章

AN - SCOPUS:105001048765

SN - 2949-754X

VL - 9

JO - Materials Today Catalysis

JF - Materials Today Catalysis

M1 - 100098

ER -

Constructing electron transport channel of SnO2/BaSO4 on g-C3N4 for enhanced visible-light-driven photocatalytic H2 production

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Constructing electron transport channel of SnO₂/BaSO₄ on g-C₃N₄ for enhanced visible-light-driven photocatalytic H₂ production