A template carbonization strategy to synthesize ordered mesoporous silica microspheres with trapped sulfonated carbon nanoparticles for efficient catalysis

Qin Yue; Minghong Wang; Jing Wei; Yonghui Deng; Tianyi Liu; Renchao Che; Bo Tu; Dongyuan Zhao

doi:10.1002/anie.201204719

A template carbonization strategy to synthesize ordered mesoporous silica microspheres with trapped sulfonated carbon nanoparticles for efficient catalysis

Qin Yue
, Minghong Wang
, Jing Wei
, Yonghui Deng
, Tianyi Liu
, Renchao Che
, Bo Tu
, Dongyuan Zhao

Fudan University

科研成果: 期刊稿件 › 文章 › 同行评审

73 引用（Scopus）

摘要

A facile template carbonization strategy has been used for the synthesis of ordered mesoporous silica microspheres with sulfonated carbon nanoparticles trapped inside by combining solvent-evaporation-induced aggregating assembly, in situ carbonization, and sulfonation treatments. The obtained SO ₃H-bearing microspheres show an excellent catalytic performance in the condensation reaction of benzaldehyde with ethylene glycol.

源语言	英语
页（从-至）	10368-10372
页数	5
期刊	Angewandte Chemie - International Edition
卷	51
期	41
DOI	https://doi.org/10.1002/anie.201204719
出版状态	已出版 - 8 10月 2012
已对外发布	是

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abstract = "A facile template carbonization strategy has been used for the synthesis of ordered mesoporous silica microspheres with sulfonated carbon nanoparticles trapped inside by combining solvent-evaporation-induced aggregating assembly, in situ carbonization, and sulfonation treatments. The obtained SO 3H-bearing microspheres show an excellent catalytic performance in the condensation reaction of benzaldehyde with ethylene glycol.",

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AU - Yue, Qin

AU - Wang, Minghong

AU - Wei, Jing

AU - Deng, Yonghui

AU - Liu, Tianyi

AU - Che, Renchao

AU - Tu, Bo

AU - Zhao, Dongyuan

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AB - A facile template carbonization strategy has been used for the synthesis of ordered mesoporous silica microspheres with sulfonated carbon nanoparticles trapped inside by combining solvent-evaporation-induced aggregating assembly, in situ carbonization, and sulfonation treatments. The obtained SO 3H-bearing microspheres show an excellent catalytic performance in the condensation reaction of benzaldehyde with ethylene glycol.

KW - block copolymers

KW - carbon nanoparticles

KW - heterogeneous catalysis

KW - mesoporous materials

KW - sulfonation

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ER -

A template carbonization strategy to synthesize ordered mesoporous silica microspheres with trapped sulfonated carbon nanoparticles for efficient catalysis

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