TY - JOUR
T1 - Two-Dimensional Transition-Metal Oxides Mn2O3Realized the Quantum Anomalous Hall Effect
AU - Li, Ping
AU - Cai, Tian Yi
N1 - Publisher Copyright:
© 2020 American Chemical Society.
PY - 2020/6/11
Y1 - 2020/6/11
N2 - The quantum anomalous Hall effect is an intriguing topological nontrivial phase arising from spontaneous magnetization and spin-orbit coupling. However, the tremendously harsh realizing requirements of the quantum anomalous Hall effects in magnetic topological insulators of Cr- or V-doped (Bi,Sb)2Te3 films hinder their practical applications. Here, we perform first-principles calculations to predict that three Mn2O3 structures are intrinsic ferromagnetic Chern insulators. Remarkably, a quantum anomalous Hall phase of Chern number C = -2 is found, and there are two corresponding gapless chiral edge states appearing inside the bulk gap. More interestingly, only a small tensile strain is needed to induce the phase transition from the Cmm2 and C222 phases to the P6/mmm phase. Meanwhile, a topological quantum phase transition from a quantum anomalous Hall phase to a trivial insulating phase can be realized. The combination of these novel properties renders the two-dimensional ferromagnet a promising platform for highly efficient electronic and spintronic devices.
AB - The quantum anomalous Hall effect is an intriguing topological nontrivial phase arising from spontaneous magnetization and spin-orbit coupling. However, the tremendously harsh realizing requirements of the quantum anomalous Hall effects in magnetic topological insulators of Cr- or V-doped (Bi,Sb)2Te3 films hinder their practical applications. Here, we perform first-principles calculations to predict that three Mn2O3 structures are intrinsic ferromagnetic Chern insulators. Remarkably, a quantum anomalous Hall phase of Chern number C = -2 is found, and there are two corresponding gapless chiral edge states appearing inside the bulk gap. More interestingly, only a small tensile strain is needed to induce the phase transition from the Cmm2 and C222 phases to the P6/mmm phase. Meanwhile, a topological quantum phase transition from a quantum anomalous Hall phase to a trivial insulating phase can be realized. The combination of these novel properties renders the two-dimensional ferromagnet a promising platform for highly efficient electronic and spintronic devices.
UR - https://www.scopus.com/pages/publications/85087840808
U2 - 10.1021/acs.jpcc.0c01308
DO - 10.1021/acs.jpcc.0c01308
M3 - 文章
AN - SCOPUS:85087840808
SN - 1932-7447
VL - 124
SP - 12705
EP - 12712
JO - Journal of Physical Chemistry C
JF - Journal of Physical Chemistry C
IS - 23
ER -