Temperature-independent thermal radiation

  • Alireza Shahsafi
  • , Patrick Roney
  • , You Zhou
  • , Zhen Zhang
  • , Yuzhe Xiao
  • , Chenghao Wan
  • , Raymond Wambold
  • , Jad Salman
  • , Zhaoning Yu
  • , Jiarui Li
  • , Jerzy T. Sadowski
  • , Riccardo Comin
  • , Shriram Ramanathan
  • , Mikhail A. Kats

Research output: Contribution to journalArticlepeer-review

118 Scopus citations

Abstract

Thermal emission is the process by which all objects at nonzero temperatures emit light and is well described by the Planck, Kirchhoff, and Stefan-Boltzmann laws. For most solids, the thermally emitted power increases monotonically with temperature in a one-to-one relationship that enables applications such as infrared imaging and noncontact thermometry. Here, we demonstrated ultrathin thermal emitters that violate this one-to-one relationship via the use of samarium nickel oxide (SmNiO3), a strongly correlated quantum material that undergoes a fully reversible, temperaturedriven solid-state phase transition. The smooth and hysteresis-free nature of this unique insulator-to-metal phase transition enabled us to engineer the temperature dependence of emissivity to precisely cancel out the intrinsic blackbody profile described by the Stefan- Boltzmann law, for both heating and cooling. Our design results in temperature-independent thermally emitted power within the long-wave atmospheric transparency window (wavelengths of 8 to 14 μm), across a broad temperature range of ~30 °C, centered around ~120 °C. The ability to decouple temperature and thermal emission opens a gateway for controlling the visibility of objects to infrared cameras and, more broadly, opportunities for quantum materials in controlling heat transfer.

Original languageEnglish
Pages (from-to)26402-26406
Number of pages5
JournalProceedings of the National Academy of Sciences of the United States of America
Volume116
Issue number52
DOIs
StatePublished - 26 Dec 2019
Externally publishedYes

Keywords

  • Heat transfer
  • Phase transition
  • Quantum materials
  • Thermal emission
  • Thermal radiation

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