Synthesis of polymer-montmorillonite nanocomposites by in situ intercalative polymerization

  • Q. H. Zeng
  • , D. Z. Wang
  • , A. B. Yu
  • , G. Q. Lu

Research output: Contribution to journalArticlepeer-review

164 Scopus citations

Abstract

Two polymer-montmorillonite (MMT) nanocomposites have been synthesized by in situ intercalative polymerization. The styrene monomer is intercalated into the interlayer space of organically modified MMT, a layered clay mineral. Upon the intercalation, the complex is subsequently polymerized in the confinement environment of the interlayer space with a free radical initiator, 2,2-azobis isobutyronitrile. The aniline monomer is also intercalated and then polymerized within the interlayer space of sodium- and copper-MMT initiated by ammonium peroxodisulphate and interlayer copper cations respectively. X-ray diffraction indicates that the MMT layers are completely dispersed in the polystyrene matrix and an exfoliated structure has been obtained. The resulting polyaniline-MMT nanocomposites show a highly ordered structure of a single polyaniline layer stacked with the MMT layers. Fourier transform infrared spectra further confirm the intercalation and formation of both polymer-MMT nanocomposites.

Original languageEnglish
Pages (from-to)549-553
Number of pages5
JournalNanotechnology
Volume13
Issue number5
DOIs
StatePublished - Oct 2002

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