Relaxor antiferroelectric-like characteristic boosting enhanced energy storage performance in eco-friendly (Bi0.5Na0.5)TiO3-based ceramics

Wenjing Shi; Leiyang Zhang; Ruiyi Jing; Qingyuan Hu; Xinyu Zeng; D. O. Alikin; V. Ya Shur; Xiaoyong Wei; Jinghui Gao; Gang Liu; Yan Yan; Li Jin

doi:10.1016/j.jeurceramsoc.2022.04.057

Relaxor antiferroelectric-like characteristic boosting enhanced energy storage performance in eco-friendly (Bi_0.5Na_0.5)TiO₃-based ceramics

Wenjing Shi
, Leiyang Zhang
, Ruiyi Jing
, Qingyuan Hu
, Xinyu Zeng
, D. O. Alikin
, V. Ya Shur
, Xiaoyong Wei
, Jinghui Gao
, Gang Liu
, Yan Yan
, Li Jin

Xi'an Jiaotong University
Southwest University
Ural Federal University

Research output: Contribution to journal › Article › peer-review

75 Scopus citations

Abstract

Ideal relaxor antiferroelectrics (RAFEs) have high field-induced polarization, low remnant polarization and very slim hysteresis, which can generate high recoverable energy storage W_rec and high energy storage efficiency η, thus attracting much attention for energy storage applications. True RAFEs, on the other hand, are extremely rare, and the majority of them contain environmentally hazardous lead. In this work, we use a viscous polymer rolling process to synthesize a novel and eco-friendly 0.65Bi_0.5Na_0.4K_0.1TiO₃-0.35[2/3SrTiO₃-1/3Bi(Mg_2/3Nb_1/3)O₃] (BNKT-ST-BMN) dielectric material, which possesses a very typical RAFE-like characteristic. As a result, this material has a high W_rec of 4.43 J/cm³ and a η of 86% at an electric felid of 290 kV/cm, as well as a high thermal stability of W_rec (>3 J/cm³) over a wide range of 30–140 °C at 250 kV/cm. Our findings suggest that the BNKT-ST-BMN material could be a potential candidate for use in energy storage pulse capacitors.

Original language	English
Pages (from-to)	4528-4538
Number of pages	11
Journal	Journal of the European Ceramic Society
Volume	42
Issue number	11
DOIs	https://doi.org/10.1016/j.jeurceramsoc.2022.04.057
State	Published - Sep 2022

Keywords

BNT-based
Eco-friendly
Energy storage
Relaxor ferroelectrics
Viscous polymer process

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10.1016/j.jeurceramsoc.2022.04.057

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Shi, W., Zhang, L., Jing, R., Hu, Q., Zeng, X., Alikin, D. O., Shur, V. Y., Wei, X., Gao, J., Liu, G., Yan, Y., & Jin, L. (2022). Relaxor antiferroelectric-like characteristic boosting enhanced energy storage performance in eco-friendly (Bi_0.5Na_0.5)TiO₃-based ceramics. Journal of the European Ceramic Society, 42(11), 4528-4538. https://doi.org/10.1016/j.jeurceramsoc.2022.04.057

@article{03fc86b1298442ecb44651ff61259002,

title = "Relaxor antiferroelectric-like characteristic boosting enhanced energy storage performance in eco-friendly (Bi0.5Na0.5)TiO3-based ceramics",

abstract = "Ideal relaxor antiferroelectrics (RAFEs) have high field-induced polarization, low remnant polarization and very slim hysteresis, which can generate high recoverable energy storage Wrec and high energy storage efficiency η, thus attracting much attention for energy storage applications. True RAFEs, on the other hand, are extremely rare, and the majority of them contain environmentally hazardous lead. In this work, we use a viscous polymer rolling process to synthesize a novel and eco-friendly 0.65Bi0.5Na0.4K0.1TiO3-0.35[2/3SrTiO3-1/3Bi(Mg2/3Nb1/3)O3] (BNKT-ST-BMN) dielectric material, which possesses a very typical RAFE-like characteristic. As a result, this material has a high Wrec of 4.43 J/cm3 and a η of 86\% at an electric felid of 290 kV/cm, as well as a high thermal stability of Wrec (>3 J/cm3) over a wide range of 30{\textendash}140 °C at 250 kV/cm. Our findings suggest that the BNKT-ST-BMN material could be a potential candidate for use in energy storage pulse capacitors.",

keywords = "BNT-based, Eco-friendly, Energy storage, Relaxor ferroelectrics, Viscous polymer process",

author = "Wenjing Shi and Leiyang Zhang and Ruiyi Jing and Qingyuan Hu and Xinyu Zeng and Alikin, \{D. O.\} and Shur, \{V. Ya\} and Xiaoyong Wei and Jinghui Gao and Gang Liu and Yan Yan and Li Jin",

note = "Publisher Copyright: {\textcopyright} 2022 Elsevier Ltd",

year = "2022",

month = sep,

doi = "10.1016/j.jeurceramsoc.2022.04.057",

language = "英语",

volume = "42",

pages = "4528--4538",

journal = "Journal of the European Ceramic Society",

issn = "0955-2219",

publisher = "Elsevier B.V.",

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Shi, W, Zhang, L, Jing, R, Hu, Q, Zeng, X, Alikin, DO, Shur, VY, Wei, X , Gao, J, Liu, G, Yan, Y & Jin, L 2022, 'Relaxor antiferroelectric-like characteristic boosting enhanced energy storage performance in eco-friendly (Bi_0.5Na_0.5)TiO₃-based ceramics', Journal of the European Ceramic Society, vol. 42, no. 11, pp. 4528-4538. https://doi.org/10.1016/j.jeurceramsoc.2022.04.057

TY - JOUR

T1 - Relaxor antiferroelectric-like characteristic boosting enhanced energy storage performance in eco-friendly (Bi0.5Na0.5)TiO3-based ceramics

AU - Shi, Wenjing

AU - Zhang, Leiyang

AU - Jing, Ruiyi

AU - Hu, Qingyuan

AU - Zeng, Xinyu

AU - Alikin, D. O.

AU - Shur, V. Ya

AU - Wei, Xiaoyong

AU - Gao, Jinghui

AU - Liu, Gang

AU - Yan, Yan

AU - Jin, Li

PY - 2022/9

Y1 - 2022/9

N2 - Ideal relaxor antiferroelectrics (RAFEs) have high field-induced polarization, low remnant polarization and very slim hysteresis, which can generate high recoverable energy storage Wrec and high energy storage efficiency η, thus attracting much attention for energy storage applications. True RAFEs, on the other hand, are extremely rare, and the majority of them contain environmentally hazardous lead. In this work, we use a viscous polymer rolling process to synthesize a novel and eco-friendly 0.65Bi0.5Na0.4K0.1TiO3-0.35[2/3SrTiO3-1/3Bi(Mg2/3Nb1/3)O3] (BNKT-ST-BMN) dielectric material, which possesses a very typical RAFE-like characteristic. As a result, this material has a high Wrec of 4.43 J/cm3 and a η of 86% at an electric felid of 290 kV/cm, as well as a high thermal stability of Wrec (>3 J/cm3) over a wide range of 30–140 °C at 250 kV/cm. Our findings suggest that the BNKT-ST-BMN material could be a potential candidate for use in energy storage pulse capacitors.

AB - Ideal relaxor antiferroelectrics (RAFEs) have high field-induced polarization, low remnant polarization and very slim hysteresis, which can generate high recoverable energy storage Wrec and high energy storage efficiency η, thus attracting much attention for energy storage applications. True RAFEs, on the other hand, are extremely rare, and the majority of them contain environmentally hazardous lead. In this work, we use a viscous polymer rolling process to synthesize a novel and eco-friendly 0.65Bi0.5Na0.4K0.1TiO3-0.35[2/3SrTiO3-1/3Bi(Mg2/3Nb1/3)O3] (BNKT-ST-BMN) dielectric material, which possesses a very typical RAFE-like characteristic. As a result, this material has a high Wrec of 4.43 J/cm3 and a η of 86% at an electric felid of 290 kV/cm, as well as a high thermal stability of Wrec (>3 J/cm3) over a wide range of 30–140 °C at 250 kV/cm. Our findings suggest that the BNKT-ST-BMN material could be a potential candidate for use in energy storage pulse capacitors.

KW - BNT-based

KW - Eco-friendly

KW - Energy storage

KW - Relaxor ferroelectrics

KW - Viscous polymer process

UR - https://www.scopus.com/pages/publications/85129343847

U2 - 10.1016/j.jeurceramsoc.2022.04.057

DO - 10.1016/j.jeurceramsoc.2022.04.057

M3 - 文章

AN - SCOPUS:85129343847

SN - 0955-2219

VL - 42

SP - 4528

EP - 4538

JO - Journal of the European Ceramic Society

JF - Journal of the European Ceramic Society

IS - 11

ER -

Relaxor antiferroelectric-like characteristic boosting enhanced energy storage performance in eco-friendly (Bi_0.5Na_0.5)TiO₃-based ceramics

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