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Recent advances in high-gravity process for multiple air pollutant control and CO2 capture and utilization: theory and practice

  • Tse Lun Chen
  • , Min Hao Yuan
  • , Yi Hung Chen
  • , Yi Bo Zhao
  • , Meihong Wang
  • , Pen Chi Chiang
  • National Sun Yat-sen University
  • China Medical University Taichung
  • National Taipei University of Technology
  • University of Minnesota Twin Cities
  • University of Sheffield
  • National Taiwan University

Research output: Contribution to journalReview articlepeer-review

Abstract

Industrial emissions containing sulfur and nitrogen oxides (SOx/NOx), fine particulate matter (PM2.5), and volatile organic compounds (VOCs) present severe environmental and health hazards. Conventional control methods, such as wet scrubbers, are often hindered by large footprints and high resource consumption. This review evaluates high-gravity rotating packed bed (HiGee-RPB) technology as a transformative solution for air purification and CO2 utilization. By generating centrifugal forces 1–3 orders of magnitude greater than Earth’s gravity, HiGee-RPB intensifies mass transfer, enabling a highly compact and versatile processing platform. Case studies highlight exceptional performance, with removal efficiencies exceeding 99% for H2S/SO2 and 90% for PM2.5, attributed to enhanced droplet filtration and unique flow patterns. Furthermore, NOx removal reaches 80–91% via oxidative absorption, while VOC treatment from sources like cooking fumes shows improvement with specialized oxidants. The review also explores CO2 emission reduction through amine-based chemical absorption and accelerated mineralization using alkaline wastes. Although challenges regarding long-term stability and accurate computational fluid dynamics (CFD) modeling remain, HiGee-RPB stands out as a robust avenue for green process intensification. Future research must integrate CFD optimization and machine learning to overcome scale-up hurdles, solidifying HiGee-RPB’s role in sustainable industrial pollution control.

Original languageEnglish
JournalJournal of Industrial and Engineering Chemistry
DOIs
StateAccepted/In press - 2026
Externally publishedYes

Keywords

  • CO absorption
  • CO mineralization
  • High-gravity rotating packed bed
  • Integrated air pollution control
  • Reactor design
  • System optimization

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