Programmed synthesis palladium supported on Fe3O4@C: An efficient and heterogeneous recyclable catalyst for one-pot reductive amination of aldehydes with nitroarenes in aqueous reaction medium

Xingchun Zhou; Xinzhe Li; Lixin Jiao; Hongfei Huo; Rong Li

doi:10.1007/s10562-015-1552-1

Programmed synthesis palladium supported on Fe₃O₄@C: An efficient and heterogeneous recyclable catalyst for one-pot reductive amination of aldehydes with nitroarenes in aqueous reaction medium

Xingchun Zhou
, Xinzhe Li
, Lixin Jiao
, Hongfei Huo
, Rong Li

Lanzhou University

Research output: Contribution to journal › Article › peer-review

16 Scopus citations

Abstract

A highly efficient Pd/Fe₃O₄@C catalytic system has been developed for direct reductive amination of carbonyl compounds with nitroarenes in aqueous reaction medium. The catalyst was characterized by TEM, XRD, XPS and VSM. It was found that the catalyst showed a high activity for the one-pot direct reductive amination of aldehydes with nitroarenes in the presence of molecular hydrogen at mild temperature. Besides, the catalyst could be recovered in a facile manner from the reaction mixture and recycled six times without obvious loss in activity.

Original language	English
Pages (from-to)	1591-1599
Number of pages	9
Journal	Catalysis Letters
Volume	145
Issue number	8
DOIs	https://doi.org/10.1007/s10562-015-1552-1
State	Published - Aug 2015
Externally published	Yes

Keywords

Aldehydes
Core-shell
Nitroarenes
One-pot direct reductive amination
Pd (0)

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10.1007/s10562-015-1552-1

Cite this

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title = "Programmed synthesis palladium supported on Fe3O4@C: An efficient and heterogeneous recyclable catalyst for one-pot reductive amination of aldehydes with nitroarenes in aqueous reaction medium",

abstract = "A highly efficient Pd/Fe3O4@C catalytic system has been developed for direct reductive amination of carbonyl compounds with nitroarenes in aqueous reaction medium. The catalyst was characterized by TEM, XRD, XPS and VSM. It was found that the catalyst showed a high activity for the one-pot direct reductive amination of aldehydes with nitroarenes in the presence of molecular hydrogen at mild temperature. Besides, the catalyst could be recovered in a facile manner from the reaction mixture and recycled six times without obvious loss in activity.",

keywords = "Aldehydes, Core-shell, Nitroarenes, One-pot direct reductive amination, Pd (0)",

author = "Xingchun Zhou and Xinzhe Li and Lixin Jiao and Hongfei Huo and Rong Li",

note = "Publisher Copyright: {\textcopyright} Springer Science+Business Media New York 2015.",

year = "2015",

month = aug,

doi = "10.1007/s10562-015-1552-1",

language = "英语",

volume = "145",

pages = "1591--1599",

journal = "Catalysis Letters",

issn = "1011-372X",

publisher = "Kluwer Academic Publishers",

number = "8",

}

Programmed synthesis palladium supported on Fe₃O₄@C: An efficient and heterogeneous recyclable catalyst for one-pot reductive amination of aldehydes with nitroarenes in aqueous reaction medium. / Zhou, Xingchun; Li, Xinzhe; Jiao, Lixin et al.
In: Catalysis Letters, Vol. 145, No. 8, 08.2015, p. 1591-1599.

Research output: Contribution to journal › Article › peer-review

TY - JOUR

T1 - Programmed synthesis palladium supported on Fe3O4@C

T2 - An efficient and heterogeneous recyclable catalyst for one-pot reductive amination of aldehydes with nitroarenes in aqueous reaction medium

AU - Zhou, Xingchun

AU - Li, Xinzhe

AU - Jiao, Lixin

AU - Huo, Hongfei

AU - Li, Rong

N1 - Publisher Copyright: © Springer Science+Business Media New York 2015.

PY - 2015/8

Y1 - 2015/8

N2 - A highly efficient Pd/Fe3O4@C catalytic system has been developed for direct reductive amination of carbonyl compounds with nitroarenes in aqueous reaction medium. The catalyst was characterized by TEM, XRD, XPS and VSM. It was found that the catalyst showed a high activity for the one-pot direct reductive amination of aldehydes with nitroarenes in the presence of molecular hydrogen at mild temperature. Besides, the catalyst could be recovered in a facile manner from the reaction mixture and recycled six times without obvious loss in activity.

AB - A highly efficient Pd/Fe3O4@C catalytic system has been developed for direct reductive amination of carbonyl compounds with nitroarenes in aqueous reaction medium. The catalyst was characterized by TEM, XRD, XPS and VSM. It was found that the catalyst showed a high activity for the one-pot direct reductive amination of aldehydes with nitroarenes in the presence of molecular hydrogen at mild temperature. Besides, the catalyst could be recovered in a facile manner from the reaction mixture and recycled six times without obvious loss in activity.

KW - Aldehydes

KW - Core-shell

KW - Nitroarenes

KW - One-pot direct reductive amination

KW - Pd (0)

UR - https://www.scopus.com/pages/publications/85019402919

U2 - 10.1007/s10562-015-1552-1

DO - 10.1007/s10562-015-1552-1

M3 - 文章

AN - SCOPUS:85019402919

SN - 1011-372X

VL - 145

SP - 1591

EP - 1599

JO - Catalysis Letters

JF - Catalysis Letters

IS - 8

ER -

Programmed synthesis palladium supported on Fe₃O₄@C: An efficient and heterogeneous recyclable catalyst for one-pot reductive amination of aldehydes with nitroarenes in aqueous reaction medium

Abstract

Keywords

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