TY - JOUR
T1 - Plasma re-activation
T2 - A promising approach to enhance chemical activity for plasma activated water
AU - Wang, Sitao
AU - Liu, Zhijie
AU - Pang, Bolun
AU - Gao, Yuting
AU - Xu, Dehui
AU - Liu, Dingxin
AU - Kong, Michael G.
N1 - Publisher Copyright:
© 2022 IOP Publishing Ltd.
PY - 2022/5/5
Y1 - 2022/5/5
N2 - Plasma activated water (PAW) is a green prospective solution for a wide range of biotechnology applications. However, the drawback for the transient chemical activity of PAW would make it lose versatility in possible applications. Herein, we propose a promising approach for plasma re-activation aimed at enhancing the chemical activity of PAW again before it entirely decays. Our results indicate that the PAW generated by re-activation displays superior physicochemical properties and higher production of RONS. Especially, the concentrations of ONOO-/O2- and H2O2 by re-activation can remarkably increase by 17.88% and 34.83% compared to the initial activation, respectively. Furthermore, the low temperature storage shows excellent synergetic effects with re-activation, indicating that the re-activation actually enhances the chemical activity of PAW to a higher level. The possible reasons for high chemical activity of PAW by plasma re-activation may be affected by the synergistic effect of multi-factors including the residual RONS in stored PAW and the lower pH value, temperatures of electrode and liquid during re-activation. This study provides good insight into the nature of liquid chemistry for PAW prepered by plasma re-activation, and demonstrates a new alternative for improving the chemical activity of PAW.
AB - Plasma activated water (PAW) is a green prospective solution for a wide range of biotechnology applications. However, the drawback for the transient chemical activity of PAW would make it lose versatility in possible applications. Herein, we propose a promising approach for plasma re-activation aimed at enhancing the chemical activity of PAW again before it entirely decays. Our results indicate that the PAW generated by re-activation displays superior physicochemical properties and higher production of RONS. Especially, the concentrations of ONOO-/O2- and H2O2 by re-activation can remarkably increase by 17.88% and 34.83% compared to the initial activation, respectively. Furthermore, the low temperature storage shows excellent synergetic effects with re-activation, indicating that the re-activation actually enhances the chemical activity of PAW to a higher level. The possible reasons for high chemical activity of PAW by plasma re-activation may be affected by the synergistic effect of multi-factors including the residual RONS in stored PAW and the lower pH value, temperatures of electrode and liquid during re-activation. This study provides good insight into the nature of liquid chemistry for PAW prepered by plasma re-activation, and demonstrates a new alternative for improving the chemical activity of PAW.
KW - biomedical application
KW - chemical activity
KW - initial plasma activation
KW - plasma activated water
KW - plasma re-activation
UR - https://www.scopus.com/pages/publications/85125439287
U2 - 10.1088/1361-6463/ac4dcd
DO - 10.1088/1361-6463/ac4dcd
M3 - 文章
AN - SCOPUS:85125439287
SN - 0022-3727
VL - 55
JO - Journal of Physics D: Applied Physics
JF - Journal of Physics D: Applied Physics
IS - 18
M1 - 185202
ER -