Physical Limit of Nonlinear Brownian Oscillators in Quantum Trap

  • Fangyuan Chen
  • , Zepu Kou
  • , Zonghuiyi Jiang
  • , Wanlin Guo
  • , Xiaofei Liu

Research output: Contribution to journalArticlepeer-review

3 Scopus citations

Abstract

Quantum trap, a quantum and thermal fluctuations-induced nonmonotonous potential, offers a chance to build up microscopic mechanical systems completely dominated by fluctuations. Here, we explore the physical limit of the effective damping ratio of the nonlinear Brownian oscillator in a quantum trap, set by the finite separation for avoiding molecular-scale effects on the trap potential and the surface confinement effect-induced diverging damping and random forces. The quasiharmonic approximations and Langevin dynamics simulations show that the lowest effective damping ratios of the suspended Au plate and Au sphere upon a Teflon coating of 10 nm can be ∼210 and ∼145, respectively, at room temperature. Perforation is proposed as an effective route to reduce the damping ratio (down to 6.4) by attenuating the surface confinement effect. An unexpected result due to the temperature dependences of dielectric function and viscosity of ethanol is a further reduced damping ratio at 400 K (1.3). The nonlinear Brownian oscillator in the quantum trap shows promise of probing near-boundary hydrodynamics at nanoscale.

Original languageEnglish
Pages (from-to)1719-1725
Number of pages7
JournalJournal of Physical Chemistry Letters
Volume15
Issue number6
DOIs
StatePublished - 15 Feb 2024
Externally publishedYes

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