Abstract
In this study, we present first-principles calculations that introduce a nonvolatile spin field effect transistor (spin-FET) utilizing a van der Waals multiferroic heterostructure, specifically VSi2N4/Sc2CO2. We demonstrate that inverting the ferroelectric polarization in a Sc2CO2 monolayer can effectively modulate the electronic states of a VSi2N4 monolayer, enabling a transition from half-metal to half-semiconductor. This transition significantly alters the electronic transport properties. Furthermore, we construct a spin-FET device based on this multiferroic heterostructure and observe that the VSi2N4/Sc2CO2-based spin-FET exhibits exceptional all-electric-controlled performance. Notably, the inversion of the Sc2CO2 ferroelectric polarization yields a substantial on-off current ratio, approximately 650%, under a minimal bias voltage of 0.02 V. Additionally, we identify a unique spatially separated spin-polarized transport phenomenon, wherein pure spin-up electrons transport exclusively through VSi2N4, and spin-down electrons through Sc2CO2. Our findings suggest a promising pathway for developing low-energy dissipation and nonvolatile FET devices.
| Original language | English |
|---|---|
| Article number | 205105 |
| Journal | Physical Review B |
| Volume | 109 |
| Issue number | 20 |
| DOIs | |
| State | Published - 15 May 2024 |
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