Néel temperature enhancement by increasing the in-plane magnetic correlation in layered inorganic-organic hybrid materials

A study was conducted to demonstrate Néel temperature enhancement by increasing the in-plane magnetic correlation in layered inorganic-organic hybrid materials. It was demonstrated that dipole-dipole interactions between the layers can lead to the establishment of long-range magnetic order in two dimensions. It was also found the critical temperature is mainly dependent on the in-plane magnetic correlation. The study also demonstrated the influence of structural diversity on the magnetic properties of the compounds used to conduct investigations. The occurrence of ferrimagnetic or canted anti-ferromagnetic order in these compounds was confirmed by the observed difference in the zero-field-cooled (ZFC) and field-cooled (FC) susceptibility.