TY - JOUR
T1 - Multitasking tartaric-acid-enabled, highly conductive, and stable MXene/conducting polymer composite for ultrafast supercapacitor
AU - Zhang, Miao
AU - Héraly, Frédéric
AU - Yi, Ming
AU - Yuan, Jiayin
N1 - Publisher Copyright:
© 2021 The Author(s)
PY - 2021/6/23
Y1 - 2021/6/23
N2 - Ti3C2Tx (MXene), a thriving member of the two-dimensional (2D) materials family, has shown increasing potential in a myriad of applications, ranging from printable electronics to energy storage and separation membranes. Nevertheless, the dilemma of its oxidative instability and the easy disintegration of its assemblies in contact with water has been restricting its real-life use. Here, we report the benefits of tartaric acid, a natural source, as a non-innocent additive in the MXene composite. In water, it can, above all, inhibit oxidation of Ti3C2Tx and hold individual components in the composite Ti3C2Tx/poly(3,4-ethylenedioxy thiophene):polystyrene sulfonate) (Ti3C2Tx/PEDOT:PSS) firmly together; equally important, it can boost 4-fold the composite's electron conductivity in comparison to the additive-free equivalent. To showcase its practical value, a tartaric-acid-treated, water-stable MXene/PEDOT:PSS conductive coating is made, which serves as electrodes for an ultrafast supercapacitor; among all 2D materials-based assemblies, the designed supercapacitor delivers, to our knowledge, the record-high performance in an alternating-current filtering application.
AB - Ti3C2Tx (MXene), a thriving member of the two-dimensional (2D) materials family, has shown increasing potential in a myriad of applications, ranging from printable electronics to energy storage and separation membranes. Nevertheless, the dilemma of its oxidative instability and the easy disintegration of its assemblies in contact with water has been restricting its real-life use. Here, we report the benefits of tartaric acid, a natural source, as a non-innocent additive in the MXene composite. In water, it can, above all, inhibit oxidation of Ti3C2Tx and hold individual components in the composite Ti3C2Tx/poly(3,4-ethylenedioxy thiophene):polystyrene sulfonate) (Ti3C2Tx/PEDOT:PSS) firmly together; equally important, it can boost 4-fold the composite's electron conductivity in comparison to the additive-free equivalent. To showcase its practical value, a tartaric-acid-treated, water-stable MXene/PEDOT:PSS conductive coating is made, which serves as electrodes for an ultrafast supercapacitor; among all 2D materials-based assemblies, the designed supercapacitor delivers, to our knowledge, the record-high performance in an alternating-current filtering application.
KW - AC line filtering
KW - MXene
KW - PEDOT:PSS
KW - conducting polymer
KW - conductive coating
KW - electrochemical capacitor
KW - stability
KW - two-dimensional materials
UR - https://www.scopus.com/pages/publications/85108409486
U2 - 10.1016/j.xcrp.2021.100449
DO - 10.1016/j.xcrp.2021.100449
M3 - 文章
AN - SCOPUS:85108409486
SN - 2666-3864
VL - 2
JO - Cell Reports Physical Science
JF - Cell Reports Physical Science
IS - 6
M1 - 100449
ER -