Abstract
An improved topology optimization method is proposed to optimize the performance and structure of the packed bed microfluidic reactor (PBMR). Dimensionless general scaling factor (GSF) is established to fully reflect the multi-physical properties of first-order isothermal catalytic reaction. Reaction performance and the flow loss are combined into a multi-objective function. Pareto algorithm is developed by introducing the weighted-sum method with weight factors ω, so Pareto frontier solution composed of optimal solutions under different ω is obtained to reveal the trade-off relationship between single-objective functions. Material density controlled by the improved polynomial function is adopted as the design variable to control the catalyst distribution. Gradient information of the design variable is updated by using the adjoint-based sensitivity analysis method, and Helmholtz filter method is adopted to solve the problems of grayscale, unclear interface, and channel fracture. The results demonstrate that the GSF can reflect the scaling behavior of the topology optimization reactor. Multi-objective functions under different ω are responded by changing the distribution of catalyst blocks and channel structure, which affects the diffusion and mixing of reactant. From the perspective of engineering application, this study provides a general and efficient new method for developing high-performance PBMRs.
| Original language | English |
|---|---|
| Pages (from-to) | 2475-2501 |
| Number of pages | 27 |
| Journal | Reaction Kinetics, Mechanisms and Catalysis |
| Volume | 135 |
| Issue number | 5 |
| DOIs | |
| State | Published - Oct 2022 |
Keywords
- Microfluidic
- Multi-objective optimization algorithm
- Packed bed microfluidic reactor
- Reaction kinetic
- Topology optimization
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