MnCO3 modified PMN-PZT piezoelectric ceramics with enhancing mechanical quality factor and low loss

Chao Wang; Li Ning; Yang Li; Fei Li

doi:10.1016/j.ceramint.2023.12.399

MnCO₃ modified PMN-PZT piezoelectric ceramics with enhancing mechanical quality factor and low loss

Chao Wang
, Li Ning
, Yang Li
, Fei Li

Faculty of Electronic and Information Engineering

Xi'an Jiaotong University

Research output: Contribution to journal › Article › peer-review

25 Scopus citations

Abstract

In this work, piezoelectric ceramics 0.125 Pb(Mg_1/3Nb_2/3)O₃-0.445PbZrO₃-0.43PbTiO₃ + x mol% MnCO₃ (abbreviated as xMn-PMN-PZT) were fabricated by the solid-state sintering method. The addition of MnCO₃ presented obvious changes in the phase structure, grain size, dielectric and piezoelectric performance. It was found that the doping of 2.5 mol% MnCO₃ can achieved the maximum mechanical quality factor Q_m ∼1806 compared to the small Q_m ∼96 for pure ceramics. Meanwhile, a moderate piezoelectric coefficient d₃₃ ∼ 260 pC/N and a high Curie temperature T_c ∼325 °C were also achieved in 2.5Mn-PMN-PZT ceramics. These excellent properties were close to the hardening effect of MnCO₃ and the formation of defect dipoles in the MC-PMN-PZT ceramics.

Original language	English
Pages (from-to)	10835-10842
Number of pages	8
Journal	Ceramics International
Volume	50
Issue number	7
DOIs	https://doi.org/10.1016/j.ceramint.2023.12.399
State	Published - 1 Apr 2024

Keywords

Acceptor and donor dopants
Electromechanical properties
Lead-based ceramics
Mechanical quality factor

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10.1016/j.ceramint.2023.12.399

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@article{4401ce38f86847c8894cc604509acc90,

title = "MnCO3 modified PMN-PZT piezoelectric ceramics with enhancing mechanical quality factor and low loss",

abstract = "In this work, piezoelectric ceramics 0.125 Pb(Mg1/3Nb2/3)O3-0.445PbZrO3-0.43PbTiO3 + x mol\% MnCO3 (abbreviated as xMn-PMN-PZT) were fabricated by the solid-state sintering method. The addition of MnCO3 presented obvious changes in the phase structure, grain size, dielectric and piezoelectric performance. It was found that the doping of 2.5 mol\% MnCO3 can achieved the maximum mechanical quality factor Qm ∼1806 compared to the small Qm ∼96 for pure ceramics. Meanwhile, a moderate piezoelectric coefficient d33 ∼ 260 pC/N and a high Curie temperature Tc ∼325 °C were also achieved in 2.5Mn-PMN-PZT ceramics. These excellent properties were close to the hardening effect of MnCO3 and the formation of defect dipoles in the MC-PMN-PZT ceramics.",

keywords = "Acceptor and donor dopants, Electromechanical properties, Lead-based ceramics, Mechanical quality factor",

author = "Chao Wang and Li Ning and Yang Li and Fei Li",

note = "Publisher Copyright: {\textcopyright} 2023",

year = "2024",

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day = "1",

doi = "10.1016/j.ceramint.2023.12.399",

language = "英语",

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T1 - MnCO3 modified PMN-PZT piezoelectric ceramics with enhancing mechanical quality factor and low loss

AU - Wang, Chao

AU - Ning, Li

AU - Li, Yang

AU - Li, Fei

PY - 2024/4/1

Y1 - 2024/4/1

N2 - In this work, piezoelectric ceramics 0.125 Pb(Mg1/3Nb2/3)O3-0.445PbZrO3-0.43PbTiO3 + x mol% MnCO3 (abbreviated as xMn-PMN-PZT) were fabricated by the solid-state sintering method. The addition of MnCO3 presented obvious changes in the phase structure, grain size, dielectric and piezoelectric performance. It was found that the doping of 2.5 mol% MnCO3 can achieved the maximum mechanical quality factor Qm ∼1806 compared to the small Qm ∼96 for pure ceramics. Meanwhile, a moderate piezoelectric coefficient d33 ∼ 260 pC/N and a high Curie temperature Tc ∼325 °C were also achieved in 2.5Mn-PMN-PZT ceramics. These excellent properties were close to the hardening effect of MnCO3 and the formation of defect dipoles in the MC-PMN-PZT ceramics.

AB - In this work, piezoelectric ceramics 0.125 Pb(Mg1/3Nb2/3)O3-0.445PbZrO3-0.43PbTiO3 + x mol% MnCO3 (abbreviated as xMn-PMN-PZT) were fabricated by the solid-state sintering method. The addition of MnCO3 presented obvious changes in the phase structure, grain size, dielectric and piezoelectric performance. It was found that the doping of 2.5 mol% MnCO3 can achieved the maximum mechanical quality factor Qm ∼1806 compared to the small Qm ∼96 for pure ceramics. Meanwhile, a moderate piezoelectric coefficient d33 ∼ 260 pC/N and a high Curie temperature Tc ∼325 °C were also achieved in 2.5Mn-PMN-PZT ceramics. These excellent properties were close to the hardening effect of MnCO3 and the formation of defect dipoles in the MC-PMN-PZT ceramics.

KW - Acceptor and donor dopants

KW - Electromechanical properties

KW - Lead-based ceramics

KW - Mechanical quality factor

UR - https://www.scopus.com/pages/publications/85182437600

U2 - 10.1016/j.ceramint.2023.12.399

DO - 10.1016/j.ceramint.2023.12.399

M3 - 文章

AN - SCOPUS:85182437600

SN - 0272-8842

VL - 50

SP - 10835

EP - 10842

JO - Ceramics International

JF - Ceramics International

IS - 7

ER -

MnCO₃ modified PMN-PZT piezoelectric ceramics with enhancing mechanical quality factor and low loss

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Keywords

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