TY - JOUR
T1 - Industrial Dry Heat Island and Dispersion of Air Pollutants Induced by Large Coal-Fired Activities
AU - Xin, Jinyuan
AU - Ren, Xinbing
AU - Ma, Yongjing
AU - Zhao, Dandan
AU - Wang, Yonghong
AU - Ye, Jianhuai
AU - Wang, Zifa
AU - Cao, Junji
AU - Vilà-Guerau de Arellano, Jordi
AU - Martin, Scot T.
N1 - Publisher Copyright:
© 2024 American Chemical Society.
PY - 2024
Y1 - 2024
N2 - Notable anthropogenic heat sources such as coal-fired plants can alter the atmospheric boundary layer structure and the pollutant dispersion, thereby affecting the local environment and microclimate. Herein, in situ measurements inside a coal-fired steel plant were performed by multiple advanced lidars from 21 May to 21 June of 2021 in Yuncheng, Shanxi Province, China. Comparing with an adjacent meteorological site, we found a prominent nighttime dry heat island overhead of the factory, which was 3-10 °C hotter and 30%-60% drier than the surrounding fields. Large-eddy simulations constrained by the measured thermal contrast suggested that the heat-island-induced circulation could upward transport factory-discharged pollutants and horizontally spread them below the residual layer top, forming a mushroom-shaped cloud. The shape, size, and pollutant loading of the cloud were highly determined by thermodynamic variables such as aerodynamic wind and anthropogenic heat flux. Furthermore, these retained residual-layer pollutants can be convected downward to the ground after sunrise through the fumigation effect, causing the peaking phenomena aboveground. These peaks were statistically evidenced to be common in major urban agglomerations in China. The study provides a new insight regarding the origins of residual-layer pollutants and highlights the needs for programming representations of coal-fired heat emissions in mesoscale air-quality models.
AB - Notable anthropogenic heat sources such as coal-fired plants can alter the atmospheric boundary layer structure and the pollutant dispersion, thereby affecting the local environment and microclimate. Herein, in situ measurements inside a coal-fired steel plant were performed by multiple advanced lidars from 21 May to 21 June of 2021 in Yuncheng, Shanxi Province, China. Comparing with an adjacent meteorological site, we found a prominent nighttime dry heat island overhead of the factory, which was 3-10 °C hotter and 30%-60% drier than the surrounding fields. Large-eddy simulations constrained by the measured thermal contrast suggested that the heat-island-induced circulation could upward transport factory-discharged pollutants and horizontally spread them below the residual layer top, forming a mushroom-shaped cloud. The shape, size, and pollutant loading of the cloud were highly determined by thermodynamic variables such as aerodynamic wind and anthropogenic heat flux. Furthermore, these retained residual-layer pollutants can be convected downward to the ground after sunrise through the fumigation effect, causing the peaking phenomena aboveground. These peaks were statistically evidenced to be common in major urban agglomerations in China. The study provides a new insight regarding the origins of residual-layer pollutants and highlights the needs for programming representations of coal-fired heat emissions in mesoscale air-quality models.
KW - anthropogenic heat
KW - coal-fired steel plant
KW - dry heat island
KW - fumigation effect
KW - residual-layer pollutants
UR - https://www.scopus.com/pages/publications/85210281184
U2 - 10.1021/acs.est.4c02300
DO - 10.1021/acs.est.4c02300
M3 - 文章
C2 - 39570810
AN - SCOPUS:85210281184
SN - 0013-936X
JO - Environmental Science and Technology
JF - Environmental Science and Technology
ER -