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In situ growth of Te-doped Cs2SnCl6scintillator composite films for X-ray imaging

  • Junnan Wang
  • , Zeyu Wang
  • , Nikolai V. Gaponenko
  • , Jindou Shi
  • , Zheyuan Da
  • , Chen Zhang
  • , Yongqiang Ji
  • , Qing Yao
  • , Youlong Xu
  • , Minqiang Wang
  • Xi'an Jiaotong University
  • Belarusian State University of Informatics and Radioelectronics

Research output: Contribution to journalArticlepeer-review

Abstract

X-ray imaging technology has been integral to numerous aspects of people's lives since its inception. With the growing demand for advanced imaging technologies, lead-free metal halide perovskites have received significant attention due to their non-toxicity, stability, and excellent optical properties. This paper investigates the scintillation behaviour of a Te doped Cs2SnCl6 scintillator composite film (CF) prepared through an innovative in situ growth strategy. This approach achieves the direct growth of Cs2SnCl6:Te micro-crystals within polymethyl methacrylate (PMMA), mitigating the issues of optical property degradation and inhomogeneous distribution that are inevitable in a conventional two-step mixing method. By controllable optimization of the doping ratio of Te, the Cs2SnCl6:Te/PMMA CFs exhibited exceptional scintillation properties under X-ray irradiation, with the detection limit reaching up to 112 nGyairs_1. In X-ray imaging applications, the Cs2SnCl6:Te 15%/PMMA CF demonstrated advanced sensitivity, producing highresolution structural images of the target object. This advancement highlights the promising potential of lead-free metal halide perovskites in the development and application of X-ray imaging technology.

Original languageEnglish
Pages (from-to)3047-3053
Number of pages7
JournalJournal of Materials Chemistry C
Volume13
Issue number6
DOIs
StatePublished - 17 Dec 2024

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