TY - JOUR
T1 - Efficient low-frequency microwave absorption and solar evaporation properties of γ-Fe2O3 nanocubes/graphene composites
AU - Wang, Fengyi
AU - Li, Xinzhe
AU - Chen, Zhihui
AU - Yu, Wei
AU - Loh, Kian Ping
AU - Zhong, Bo
AU - Shi, Yumeng
AU - Xu, Qing Hua
N1 - Publisher Copyright:
© 2020 Elsevier B.V.
PY - 2021/2/1
Y1 - 2021/2/1
N2 - Microwave absorption and solar evaporation have attracted significant interests and great advances have been achieved in the elimination of electromagnetic radiation pollution and production of fresh water. However, enhancing low-frequency microwave absorption properties as well as mass production of cheap solar evaporators with high evaporation rate are still facing many challenges. Herein, γ-Fe2O3 nanocubes/graphene (GFC) composites were prepared by a facile one-step solvothermal method. GFC was mixed with paraffin to study its microwave absorption properties. The minimum reflection loss (RL) value of -59.3 dB at 2.4 GHz was achieved by GFC, while the RL value also reached -57.2 dB at 5.12 GHz with a thickness of 5.30 mm. Moreover, under matching frequency and thickness a good absorption performance (RL ≤ -17.2 dB) from 2.00 to 18.00 GHz was obtained, in particular, RL < -30.0 dB in S band and RL < -26.0 dB in C band. Excellent microwave absorption performance of GFC in S and C band is mainly attributed to high impedance matching, which suggests the direction for development of high-efficient low-frequency microwave absorption materials. Interfacial solar evaporator was also prepared by using GFC modified scouring sponge as light absorption layer, which has > 97% absorption in entire solar spectrum range. Its evaporation rate (3.490 kg m-2h−1) is 5.1 times larger than that of pure water under the same condition, which shows great potential applications in desalination, water purification and energy generation.
AB - Microwave absorption and solar evaporation have attracted significant interests and great advances have been achieved in the elimination of electromagnetic radiation pollution and production of fresh water. However, enhancing low-frequency microwave absorption properties as well as mass production of cheap solar evaporators with high evaporation rate are still facing many challenges. Herein, γ-Fe2O3 nanocubes/graphene (GFC) composites were prepared by a facile one-step solvothermal method. GFC was mixed with paraffin to study its microwave absorption properties. The minimum reflection loss (RL) value of -59.3 dB at 2.4 GHz was achieved by GFC, while the RL value also reached -57.2 dB at 5.12 GHz with a thickness of 5.30 mm. Moreover, under matching frequency and thickness a good absorption performance (RL ≤ -17.2 dB) from 2.00 to 18.00 GHz was obtained, in particular, RL < -30.0 dB in S band and RL < -26.0 dB in C band. Excellent microwave absorption performance of GFC in S and C band is mainly attributed to high impedance matching, which suggests the direction for development of high-efficient low-frequency microwave absorption materials. Interfacial solar evaporator was also prepared by using GFC modified scouring sponge as light absorption layer, which has > 97% absorption in entire solar spectrum range. Its evaporation rate (3.490 kg m-2h−1) is 5.1 times larger than that of pure water under the same condition, which shows great potential applications in desalination, water purification and energy generation.
KW - Graphene
KW - Impedance matching
KW - Interfacial water evaporation
KW - Microwave absorption
KW - γ-FeO nanocubes
UR - https://www.scopus.com/pages/publications/85089835467
U2 - 10.1016/j.cej.2020.126676
DO - 10.1016/j.cej.2020.126676
M3 - 文章
AN - SCOPUS:85089835467
SN - 1385-8947
VL - 405
JO - Chemical Engineering Journal
JF - Chemical Engineering Journal
M1 - 126676
ER -