Effect of non-Thermal plasma on carbon dioxide reforming of methane to hydrogen

Hongxia Liu; Dingmeng Guo; Xin Ma; Ya Wang; Jinzhuo Xie

doi:10.1680/jener.19.00030

Effect of non-Thermal plasma on carbon dioxide reforming of methane to hydrogen

Hongxia Liu
, Dingmeng Guo
, Xin Ma
, Ya Wang
, Jinzhuo Xie

School of Energy and Power Engineering

Xi'an Jiaotong University

Research output: Contribution to journal › Article › peer-review

5 Scopus citations

Abstract

A method of hydrogen production from greenhouse gases by non-thermal plasma was studied. The effect of plasma on the reforming of methane and carbon dioxide into hydrogen was analyzed as functions of different parameters including power input, electrode gaps, total gas fluxes and methane/carbon dioxide ratios in customized single and double dielectric reactors. Results showed that higher power input, smaller electrode gap and total gas flux would contribute to better performance of reforming. Based on the results of Fourier transform infrared spectroscopy and emission spectrum analysis, the mechanism of different reforming products such as carbon monoxide, hydrogen, other organic by-products and carbon deposition is discussed based on numerous free radicals including ·C, ·CH_x, ·CO, ·H, and ·O in the discharge zone.

Original language	English
Pages (from-to)	67-78
Number of pages	12
Journal	Proceedings of Institution of Civil Engineers: Energy
Volume	174
Issue number	2
DOIs	https://doi.org/10.1680/jener.19.00030
State	Published - May 2021

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10.1680/jener.19.00030

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title = "Effect of non-Thermal plasma on carbon dioxide reforming of methane to hydrogen",

abstract = "A method of hydrogen production from greenhouse gases by non-thermal plasma was studied. The effect of plasma on the reforming of methane and carbon dioxide into hydrogen was analyzed as functions of different parameters including power input, electrode gaps, total gas fluxes and methane/carbon dioxide ratios in customized single and double dielectric reactors. Results showed that higher power input, smaller electrode gap and total gas flux would contribute to better performance of reforming. Based on the results of Fourier transform infrared spectroscopy and emission spectrum analysis, the mechanism of different reforming products such as carbon monoxide, hydrogen, other organic by-products and carbon deposition is discussed based on numerous free radicals including ·C, ·CHx, ·CO, ·H, and ·O in the discharge zone.",

author = "Hongxia Liu and Dingmeng Guo and Xin Ma and Ya Wang and Jinzhuo Xie",

year = "2021",

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doi = "10.1680/jener.19.00030",

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T1 - Effect of non-Thermal plasma on carbon dioxide reforming of methane to hydrogen

AU - Liu, Hongxia

AU - Guo, Dingmeng

AU - Ma, Xin

AU - Wang, Ya

AU - Xie, Jinzhuo

PY - 2021/5

Y1 - 2021/5

N2 - A method of hydrogen production from greenhouse gases by non-thermal plasma was studied. The effect of plasma on the reforming of methane and carbon dioxide into hydrogen was analyzed as functions of different parameters including power input, electrode gaps, total gas fluxes and methane/carbon dioxide ratios in customized single and double dielectric reactors. Results showed that higher power input, smaller electrode gap and total gas flux would contribute to better performance of reforming. Based on the results of Fourier transform infrared spectroscopy and emission spectrum analysis, the mechanism of different reforming products such as carbon monoxide, hydrogen, other organic by-products and carbon deposition is discussed based on numerous free radicals including ·C, ·CHx, ·CO, ·H, and ·O in the discharge zone.

AB - A method of hydrogen production from greenhouse gases by non-thermal plasma was studied. The effect of plasma on the reforming of methane and carbon dioxide into hydrogen was analyzed as functions of different parameters including power input, electrode gaps, total gas fluxes and methane/carbon dioxide ratios in customized single and double dielectric reactors. Results showed that higher power input, smaller electrode gap and total gas flux would contribute to better performance of reforming. Based on the results of Fourier transform infrared spectroscopy and emission spectrum analysis, the mechanism of different reforming products such as carbon monoxide, hydrogen, other organic by-products and carbon deposition is discussed based on numerous free radicals including ·C, ·CHx, ·CO, ·H, and ·O in the discharge zone.

UR - https://www.scopus.com/pages/publications/85106559575

U2 - 10.1680/jener.19.00030

DO - 10.1680/jener.19.00030

M3 - 文章

AN - SCOPUS:85106559575

SN - 1751-4223

VL - 174

SP - 67

EP - 78

JO - Proceedings of Institution of Civil Engineers: Energy

JF - Proceedings of Institution of Civil Engineers: Energy

IS - 2

ER -

Effect of non-Thermal plasma on carbon dioxide reforming of methane to hydrogen

Abstract

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