Cyclic redox strategy for sustainable recovery of lithium ions from spent lithium iron phosphate batteries

Yushuo Li; Xiangpeng Kong; Xiaofeng Liu; Shen Wang; Bo Wen; Shubing Miao; Qiang Rong; Guorui Yang; Shujiang Ding

doi:10.1016/j.matlet.2024.136779

Cyclic redox strategy for sustainable recovery of lithium ions from spent lithium iron phosphate batteries

Yushuo Li
, Xiangpeng Kong
, Xiaofeng Liu
, Shen Wang
, Bo Wen
, Shubing Miao
, Qiang Rong
, Guorui Yang
, Shujiang Ding

Xi'an Jiaotong University
Hunan Desay Battery Co. LTD

Research output: Contribution to journal › Article › peer-review

4 Scopus citations

Abstract

The growth of spent lithium-ion batteries requires a green recycling method. This paper presents an innovative hydrometallurgical approach in light of redox flow batteries, which employed Fe³⁺/Fe²⁺ as regenerative redox mediator to selectively extract Li⁺ from LiFePO₄. In contrast to the conventional method in which the oxidizer is disposable, the present scheme allows for the recycling of the oxidizer, which demonstrates the advantages of environmentally friendly, low cost and higher extraction rate, offering a novel approach to recycling spent batteries.

Original language	English
Article number	136779
Journal	Materials Letters
Volume	369
DOIs	https://doi.org/10.1016/j.matlet.2024.136779
State	Published - 15 Aug 2024

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

SDG 7 Affordable and Clean Energy

Keywords

Energy storage and conversion
Metallurgy
Oxidation

Access to Document

10.1016/j.matlet.2024.136779

Cite this

@article{77d6b3dbffd549a3878656a0b0395019,

title = "Cyclic redox strategy for sustainable recovery of lithium ions from spent lithium iron phosphate batteries",

abstract = "The growth of spent lithium-ion batteries requires a green recycling method. This paper presents an innovative hydrometallurgical approach in light of redox flow batteries, which employed Fe3+/Fe2+ as regenerative redox mediator to selectively extract Li+ from LiFePO4. In contrast to the conventional method in which the oxidizer is disposable, the present scheme allows for the recycling of the oxidizer, which demonstrates the advantages of environmentally friendly, low cost and higher extraction rate, offering a novel approach to recycling spent batteries.",

keywords = "Energy storage and conversion, Metallurgy, Oxidation",

author = "Yushuo Li and Xiangpeng Kong and Xiaofeng Liu and Shen Wang and Bo Wen and Shubing Miao and Qiang Rong and Guorui Yang and Shujiang Ding",

note = "Publisher Copyright: {\textcopyright} 2024",

year = "2024",

month = aug,

day = "15",

doi = "10.1016/j.matlet.2024.136779",

language = "英语",

volume = "369",

journal = "Materials Letters",

issn = "0167-577X",

publisher = "Elsevier B.V.",

}

TY - JOUR

T1 - Cyclic redox strategy for sustainable recovery of lithium ions from spent lithium iron phosphate batteries

AU - Li, Yushuo

AU - Kong, Xiangpeng

AU - Liu, Xiaofeng

AU - Wang, Shen

AU - Wen, Bo

AU - Miao, Shubing

AU - Rong, Qiang

AU - Yang, Guorui

AU - Ding, Shujiang

PY - 2024/8/15

Y1 - 2024/8/15

N2 - The growth of spent lithium-ion batteries requires a green recycling method. This paper presents an innovative hydrometallurgical approach in light of redox flow batteries, which employed Fe3+/Fe2+ as regenerative redox mediator to selectively extract Li+ from LiFePO4. In contrast to the conventional method in which the oxidizer is disposable, the present scheme allows for the recycling of the oxidizer, which demonstrates the advantages of environmentally friendly, low cost and higher extraction rate, offering a novel approach to recycling spent batteries.

AB - The growth of spent lithium-ion batteries requires a green recycling method. This paper presents an innovative hydrometallurgical approach in light of redox flow batteries, which employed Fe3+/Fe2+ as regenerative redox mediator to selectively extract Li+ from LiFePO4. In contrast to the conventional method in which the oxidizer is disposable, the present scheme allows for the recycling of the oxidizer, which demonstrates the advantages of environmentally friendly, low cost and higher extraction rate, offering a novel approach to recycling spent batteries.

KW - Energy storage and conversion

KW - Metallurgy

KW - Oxidation

UR - https://www.scopus.com/pages/publications/85195188689

U2 - 10.1016/j.matlet.2024.136779

DO - 10.1016/j.matlet.2024.136779

M3 - 文章

AN - SCOPUS:85195188689

SN - 0167-577X

VL - 369

JO - Materials Letters

JF - Materials Letters

M1 - 136779

ER -

Cyclic redox strategy for sustainable recovery of lithium ions from spent lithium iron phosphate batteries

Abstract

UN SDGs

Keywords

Access to Document

Other files and links

Fingerprint

Cite this