TY - JOUR
T1 - Bridged Carbon Fabric Membrane with Boosted Performance in AC Line-Filtering Capacitors
AU - Zhang, Miao
AU - Dong, Kang
AU - Saeedi Garakani, Sadaf
AU - Khorsand Kheirabad, Atefeh
AU - Manke, Ingo
AU - Wu, Mingmao
AU - Wang, Hong
AU - Qu, Liangti
AU - Yuan, Jiayin
N1 - Publisher Copyright:
© 2022 The Authors. Advanced Science published by Wiley-VCH GmbH.
PY - 2022/3/4
Y1 - 2022/3/4
N2 - High-frequency responsive capacitors with lightweight, flexibility, and miniaturization are among the most vital circuit components because they can be readily incorporated into various portable devices to smooth out the ripples for circuits. Electrode materials no doubt are at the heart of such devices. Despite tremendous efforts and recent advances, the development of flexible and scalable high-frequency responsive capacitor electrodes with superior performance remains a great challenge. Herein, a straightforward and technologically relevant method is reported to manufacture a carbon fabric membrane “glued” by nitrogen-doped nanoporous carbons produced through a polyelectrolyte complexation-induced phase separation strategy. The as-obtained flexible carbon fabric bearing a unique hierarchical porous structure, and high conductivity as well as robust mechanical properties, serves as the free-standing electrode materials of electrochemical capacitors. It delivers an ultrahigh specific areal capacitance of 2632 µF cm−2 at 120 Hz with an excellent alternating current line filtering performance, fairly higher than the state-of-the-art commercial ones. Together, this system offers the potential electrode material to be scaled up for AC line-filtering capacitors at industrial levels.
AB - High-frequency responsive capacitors with lightweight, flexibility, and miniaturization are among the most vital circuit components because they can be readily incorporated into various portable devices to smooth out the ripples for circuits. Electrode materials no doubt are at the heart of such devices. Despite tremendous efforts and recent advances, the development of flexible and scalable high-frequency responsive capacitor electrodes with superior performance remains a great challenge. Herein, a straightforward and technologically relevant method is reported to manufacture a carbon fabric membrane “glued” by nitrogen-doped nanoporous carbons produced through a polyelectrolyte complexation-induced phase separation strategy. The as-obtained flexible carbon fabric bearing a unique hierarchical porous structure, and high conductivity as well as robust mechanical properties, serves as the free-standing electrode materials of electrochemical capacitors. It delivers an ultrahigh specific areal capacitance of 2632 µF cm−2 at 120 Hz with an excellent alternating current line filtering performance, fairly higher than the state-of-the-art commercial ones. Together, this system offers the potential electrode material to be scaled up for AC line-filtering capacitors at industrial levels.
KW - alternating current line filtering
KW - phase angle
KW - poly(ionic liquid)
KW - porous carbon membrane
UR - https://www.scopus.com/pages/publications/85123168721
U2 - 10.1002/advs.202105072
DO - 10.1002/advs.202105072
M3 - 文章
C2 - 35060354
AN - SCOPUS:85123168721
SN - 2198-3844
VL - 9
JO - Advanced Science
JF - Advanced Science
IS - 7
M1 - 2105072
ER -