Abstract
With its generality and practicality, the combination of partial charging curves and machine learning (ML) for battery capacity estimation has attracted widespread attention. However, a clear classification, fair comparison, and performance rationalization of these methods are lacking, due to the scattered existing studies. To address these issues, we develop 20 capacity estimation methods from three perspectives: charging sequence construction, input forms, and ML models. 22,582 charging curves are generated from 44 cells with different battery chemistry and operating conditions to validate the performance. Through comprehensive and unbiased comparison, the long short-term memory (LSTM) based neural network exhibits the best accuracy and robustness. Across all 6503 tested samples, the mean absolute percentage error (MAPE) for capacity estimation using LSTM is 0.61%, with a maximum error of only 3.94%. Even with the addition of 3 mV voltage noise or the extension of sampling intervals to 60 s, the average MAPE remains below 2%. Furthermore, the charging sequences are provided with physical explanations related to battery degradation to enhance confidence in their application. Recommendations for using other competitive methods are also presented. This work provides valuable insights and guidance for estimating battery capacity based on partial charging curves.
| Original language | English |
|---|---|
| Pages (from-to) | 409-420 |
| Number of pages | 12 |
| Journal | Journal of Energy Chemistry |
| Volume | 88 |
| DOIs | |
| State | Published - Jan 2024 |
UN SDGs
This output contributes to the following UN Sustainable Development Goals (SDGs)
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SDG 7 Affordable and Clean Energy
Keywords
- Capacity estimation
- Data-driven
- Lithium-ion battery
- Partial charging curves
- Sampling frequency
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